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No, python is a programming(not designing ) language, so the only use I can find is program functionality. On computer, you can do Tkinter interfaces with a python module, but Tkinter GUIs are very simple.
IDK the best GUI language. If you think HTML, you're 50 by 50 right. It's a web programming language, but still can be used for simple pages and even simple games.
But HTML mostly isn't needed if you mean app GUI.